U.S. Geological Survey Open-File Report 09-0346
Trends in Precipitation Chemistry in the United States, 1983-1994: An Analysis of the Effects in 1995 of Phase I of the Clean Air Act Amendments of 1990, Title IV

Table A.4. Estimated changes in concentrations (µeq/L and percent) of individual ions in preciptation from 1983 through 1994.


               Hydrogen Ion          Sulfate            Nitrate            Chloride
             _________________  _________________  _________________  _________________
              Change   Percent   Change   Percent   Change   Percent   Change   Percent
Region Site   (µeq/L)  Change    (µeq/L)  Change    (µeq/L)  Change    (µeq/L)  Change
---------------------------------------------------------------------------------------
 NE    il11   -7.686*  -15.146   -7.399*  -12.988    0.614     2.645   -0.304    -7.999
       il18   -3.985   -11.841   -7.341   -14.694    2.502    10.677   -0.297    -8.372
       il19   -9.866*  -21.811  -11.533*  -18.528   -2.841    -9.851   -0.662   -12.516
       il35    2.767     7.652   -4.951   -11.514   -0.483    -2.725   -0.434    -9.467
       il63    0.376     0.918   -6.282*  -12.542    0.453     2.477   -0.417    -7.845
       in20   -4.035    -8.281  -15.255*  -24.788   -2.623    -9.024   -1.348*  -30.916
       in22   -0.512    -1.087    4.127     7.892    6.584*   38.812   -0.862   -15.839
       in34  -10.301*  -24.467   -7.957*  -13.028   -0.582    -2.099   -0.548   -10.859
       in41   -8.060*  -16.298   -9.104*  -15.201   -3.538   -12.701   -1.183*  -26.376
       ky03   -3.520    -8.022   -2.112    -4.687    0.300     1.643   -0.926   -21.075
       ky22   -6.620*  -16.509  -10.151*  -24.279   -3.374*  -17.747   -1.683*  -42.701
       ky35   -7.343   -15.074   -6.359   -12.972   -4.606   -20.336   -0.858*  -23.836
       ky38   -1.938    -5.723   -2.689    -7.176    1.371     8.766   -0.189    -4.259
       ma01    5.106    16.724   -0.897    -2.464    4.663    32.617    0.014     0.018
       ma08   -4.251    -9.625   -8.162   -20.377   -0.525    -2.401   -1.042   -14.949
       ma13  -10.129*  -19.810   -6.033   -12.854    1.974    11.324   -5.008*  -26.769
       md03   -0.578    -0.992   -2.749    -5.012   -0.361    -1.335   -2.241   -26.317
       md13   -5.303   -10.354   -5.893   -11.846   -1.802    -7.533   -2.262   -17.265
       me00   -4.764   -15.680   -4.307   -14.859    1.987    14.214   -0.962   -21.648
       me02    1.368     4.221   -2.525    -8.417    3.982    30.197   -1.056   -17.766
       me09    1.201     4.525   -1.749    -7.315    2.448    20.011   -0.592   -17.770
       mi09   -6.432*  -17.506   -8.165*  -20.477   -0.722    -2.755   -0.412   -14.961
       mi26   -8.570*  -19.196  -13.327*  -25.085   -2.917   -10.155   -0.675*  -16.933
       mi53   -8.420*  -20.803   -6.702*  -15.067    0.039     0.129   -0.624   -16.456
       mi98  -10.775*  -28.061  -10.626*  -26.188   -2.387    -9.054   -0.621*  -21.717
       mi99   -2.909   -13.226   -5.725*  -20.057    1.018     5.908   -0.680*  -25.718
       nh02   -2.791    -6.397   -4.967   -13.535    1.505     7.255   -0.572   -14.216
       nj99   -3.318    -6.798   -0.765    -1.668    0.764     3.339   -1.511   -13.467
       ny08   -9.416*  -14.354   -7.970   -12.598   -2.883    -8.736   -0.914*  -21.282
       ny10  -10.530*  -16.301  -17.690*  -27.125   -1.567    -4.840   -1.610*  -31.584
       ny20   -1.749    -4.049   -5.130   -13.523   -0.957    -4.208   -0.898*  -30.867
       ny52  -10.207*  -16.442  -10.778*  -18.542   -3.510    -9.759   -1.441*  -28.898
       ny65    1.053     1.965   -2.843    -5.709    0.734     2.925   -0.321   -10.548
       ny68    1.520     3.147   -2.342    -5.447    1.944     8.287   -0.204    -5.117
       ny98   -9.057*  -20.861  -10.998*  -26.653   -2.680   -12.646   -0.421   -19.200
       ny99   -5.387    -9.590   -7.092   -14.591   -3.960   -14.863    1.353    13.360
       oh09   -6.053   -10.329   -6.832   -11.075   -1.333    -5.438   -0.248    -6.085
       oh17   -0.969    -1.710   -2.545    -4.120    0.666     2.279   -0.176    -4.294
       oh49   -0.756    -1.105   -2.783    -3.974    1.829     6.616   -0.372    -7.350
       oh71   -4.392    -7.443   -4.850    -7.544   -1.437    -4.825   -0.507   -11.768
       pa15  -14.989*  -21.166  -12.499*  -19.872   -6.720*  -20.746   -1.129*  -22.594
       pa29   -9.636*  -14.013   -7.594   -12.269   -1.536    -5.188   -0.607   -14.294
       pa42   -8.500   -12.824  -10.300   -17.041   -4.143   -13.111   -0.582   -11.965
       pa72   -9.461   -15.924  -10.793   -20.984   -3.281   -11.338   -1.407   -20.722
       va00   -7.214   -13.640   -5.626   -11.670   -4.515   -17.906   -0.266    -4.484
       va13    2.911     8.700    0.358     0.979    1.975    12.522   -0.637   -16.887
       va28   -7.092*  -20.044   -9.270*  -25.231   -2.978   -19.344   -1.744*  -40.299
       vt01    8.432    20.283    2.704     6.920    5.932*   27.040    0.006     0.156
       vt99   -1.224    -2.814   -1.919    -5.069    1.305     5.476   -0.285   -11.520
       wi28  -11.771*  -42.646  -15.264*  -36.309   -3.314   -13.128   -1.065*  -31.059
       wi36   -4.346   -21.102   -7.405*  -26.619    0.809     4.394   -0.490*  -22.549
       wi37   -3.601   -21.947   -8.438*  -28.470    0.106     0.513   -0.708*  -26.963
       wi99   -4.221   -12.110  -10.748*  -21.866   -0.767    -2.828   -1.298*  -30.946
       wv04   -9.779*  -20.006  -14.136*  -29.762   -2.738   -13.023   -1.051*  -29.310
       wv18    4.110     7.389    1.295     2.346    1.465     5.885   -0.526*  -14.401
       --------------------------------------------------------------------------------
 SE    al10    2.143     9.984   -5.903*  -20.977   -1.290   -10.714   -2.055   -23.655
       al99   -5.991   -18.741   -9.508   -24.084    0.653     5.054   -0.485    -8.509
       fl03    1.497     6.931   -0.609    -2.593    2.710    28.850   -3.351   -19.705
       fl11    0.237     2.634   -0.547    -3.498    1.821    29.430    4.736    14.864
       fl14   -1.789    -9.171   -1.232    -6.621    0.994    12.287   -1.292   -10.509
       fl41    2.449    16.627   -1.530    -7.376    1.457    14.562   -2.252   -11.308
       ga20   -4.463   -19.522   -4.582   -18.508    0.851     8.333   -0.435    -4.228
       ga41   -1.391    -5.184   -4.791   -15.644   -0.924    -7.665   -2.242*  -28.732
       ga50    2.191    13.005   -2.074   -10.257    1.138    12.498   -1.729   -17.618
       ms10   -1.659    -8.801   -7.330*  -28.084   -0.567    -4.808   -1.851   -22.186
       ms30   -3.798   -17.237   -8.083*  -32.691   -1.598   -13.303   -0.966   -14.970
       nc03   -4.601   -14.697   -7.455*  -21.790   -1.600   -10.566   -2.833   -19.753
       nc25   -3.844   -13.803   -7.943*  -25.356   -1.415   -12.123   -0.652   -13.166
       nc34   -1.488    -3.952   -2.208    -5.265   -1.237    -6.805   -0.122    -1.796
       nc36    8.063*   28.991    5.665    20.077    4.986*   39.317    0.604     6.240
       nc41   -6.281   -20.078   -6.814   -19.045   -1.891   -11.698   -2.595   -24.568
       sc06   -3.544   -12.182   -6.800   -20.781    1.662    15.666   -0.283    -2.198
       tn00   -2.485    -5.240   -9.982*  -19.532   -0.920    -5.246   -1.490*  -25.053
       tn11   -1.085    -3.348   -4.202   -12.141   -1.175    -7.904   -0.633   -18.836
       tn14    2.792    12.875    1.594     6.843    3.049*   26.288   -1.220   -23.820
---------------------------------------------------------------------------------------
* Annual trend was significant (p<0.05).
---------------------------------------------------------------------------------------

               Hydrogen Ion          Sulfate            Nitrate            Chloride
             _________________  _________________  _________________  _________________
              Change   Percent   Change   Percent   Change   Percent   Change   Percent
Region Site   (µeq/L)  Change    (µeq/L)  Change    (µeq/L)  Change    (µeq/L)  Change
---------------------------------------------------------------------------------------
 West  ak03   -1.022   -14.915   -1.370   -30.398    1.123*   83.978   -0.214    -9.961
       ar02    1.255     8.259   -3.770   -15.253    0.569     4.656    0.373     5.956
       ar03   -2.009    -8.834   -3.448   -12.736   -0.792    -5.524    0.041     0.690
       ar16    1.508     7.933   -2.019    -7.981    0.113     0.845   -0.837*  -18.896
       ar27   -2.622   -19.467   -6.637*  -24.419   -1.073    -7.159   -0.596   -13.228
       az03   -0.940   -13.464   -6.973*  -38.732    0.922     6.923   -1.160   -26.798
       az06   -0.495    -6.783   -5.676   -23.647   -2.856   -15.509   -1.780    -8.939
       az99  -10.822*  -53.165  -14.347*  -45.606   -0.349    -2.847   -0.249    -6.200
       ca42  -11.358*  -53.773   -8.851*  -37.800   -9.304   -27.569   -2.210   -16.163
       ca45   -1.368*  -26.118   -2.668*  -39.510    1.276    34.085   -3.589   -31.664
       ca75   -2.200*  -45.562   -3.530   -27.754    4.507    31.240   -1.262   -29.208
       ca88   -0.780*  -41.635   -4.862*  -24.974    0.496     2.289   -1.824   -19.206
       ca98   -4.293   -40.056   -8.858*  -52.688   -4.668   -24.167   -3.388*  -50.924
       ca99   -1.280   -16.603   -3.463   -30.993    1.267     8.220   -0.681   -16.069
       co00   -1.490   -23.973   -5.813*  -32.143   -1.567   -14.234   -1.304*  -39.688
       co01   -2.173*  -46.153   -1.036    -5.717   -1.227    -6.269   -1.196   -31.578
       co02    0.335     2.833    0.020     0.153    5.417*   50.805   -0.349   -14.023
       co15   -0.334    -2.883   -3.255   -18.829    1.818    12.954   -0.849*  -27.540
       co19   -1.013    -9.279   -5.052*  -30.500    3.841*   26.347   -0.335   -12.519
       co21    0.273     1.959   -2.449   -15.214    2.670    14.997   -0.614*  -24.087
       co22   -3.206*  -37.967   -5.681*  -30.530   -1.897    -9.519   -0.910*  -31.359
       co97    1.221     8.901    4.472*   33.368    6.188*   89.920    0.331    20.233
       co98   -1.888   -16.570   -4.954*  -33.894   -0.101    -0.904   -0.733*  -29.766
       co99   -3.770   -23.072   -4.950*  -20.925    0.772     5.251   -0.312   -11.563
       ia08    2.591    19.465   -2.419    -6.566    4.958    23.033   -0.559   -18.285
       ia23   -5.167   -29.378   -6.180   -18.327    5.239    30.921   -0.378   -12.636
       id03   -0.252    -4.943   -3.098   -25.400    3.543    37.135   -1.609*  -33.508
       id11   -2.666*  -44.656    0.068     0.781    5.569*   67.397   -0.566   -15.050
       id15   -1.878   -28.189   -0.812   -13.771    2.013*   33.745   -0.196    -8.960
       ks07   -2.295   -12.816   -5.060   -16.436    0.273     1.643   -1.342*  -31.547
       ks31   -2.643   -18.426   -1.482    -5.396    2.627    13.603   -0.479   -14.458
       ks32   -1.086   -23.241   -1.124    -5.930    5.625*   35.999   -0.636   -22.278
       la12   -0.949    -5.888   -4.621*  -19.368   -0.716    -5.964   -3.431   -18.502
       la30    1.570     9.314   -4.821*  -19.437   -0.972    -7.885   -3.627*  -25.201
       mn16   -4.450   -29.933  -10.654*  -42.126   -2.785   -14.456   -1.107*  -42.338
       mn18   -0.302    -2.212   -4.730*  -24.123   -0.128    -0.849   -0.683*  -33.065
       mn23   -0.520    -5.654   -2.678   -13.208    2.781    16.302   -0.158    -8.031
       mn27   -1.796   -24.658   -9.767*  -31.578   -2.583   -10.399   -1.274*  -38.745
       mo03   -7.190*  -26.516  -10.297*  -27.416   -1.873    -9.394   -0.696*  -18.475
       mo05   -1.947    -6.750   -4.775   -13.682   -0.911    -5.108   -0.791   -16.930
       mt00   -0.354    -4.459   -2.615   -17.484    1.717    16.942   -0.973*  -35.923
       mt05   -0.734    -8.229   -2.424*  -26.097    0.579     9.978   -0.830*  -39.579
       mt07    0.034     0.399   -1.999   -19.297    1.351    20.739   -0.833*  -35.492
       mt13   -1.504   -19.481   -0.118    -0.583    2.579    21.649   -1.044*  -35.820
       nd07   -2.101   -22.814   -6.035*  -28.930   -0.923    -6.725   -0.820*  -33.175
       nd08   -1.248   -19.054   -3.521   -18.105    0.287     1.664   -0.630   -24.361
       nd11   -1.370   -26.814   -8.990*  -32.615   -4.593   -17.776   -1.135*  -35.893
       ne15   -3.747*  -45.079   -7.262*  -20.967    1.375     6.472   -0.943*  -30.323
       nm07   -1.156    -9.489   -5.616*  -29.176   -0.002    -0.016   -1.477*  -45.922
       nm08   -3.507*  -38.893   -4.793   -23.604    1.336    14.364   -1.067   -31.244
       nm09   -4.021*  -27.596   -5.412*  -28.396   -0.533    -4.051   -1.028*  -32.435
       nm12   -2.223   -25.067    2.855    23.329   10.544*  173.269   -0.970   -30.587
       ok00   -1.164   -11.527   -4.835   -17.999   -0.117    -0.606   -3.205*  -44.679
       ok17   -1.348   -12.237   -6.101   -23.088   -0.509    -3.178   -1.881*  -34.658
       or02   -0.936   -16.976   -2.351*  -28.856    1.114*   72.324  -10.162   -30.627
       or09   -1.233   -14.897   -0.191    -3.497    3.604*   74.343   -2.107*  -54.711
       or10   -0.438    -6.924   -1.746*  -31.201    1.315*   50.277   -2.088   -26.522
       or18   -2.900*  -31.972   -0.353    -7.570    2.003    43.798   -0.608*  -28.563
       or97   -1.660*  -28.635   -2.293*  -26.831    1.277*   34.775   -1.433    -9.597
       or98   -1.266   -14.949   -1.718*  -17.859    0.792    14.884   -1.298    -9.086
       sd08   -1.409   -18.721   -4.149   -26.274   -0.207    -1.483   -0.704*  -29.630
       sd99   -4.137*  -63.535   -6.430   -27.994   -0.973    -5.266   -0.508   -20.043
       tx03    2.599    25.544   -0.924    -3.236    1.068     8.012   -2.955   -12.219
       tx04   -0.453   -10.481    3.092    15.899    5.192*   60.543   -0.441   -12.040
       tx10    2.363    17.542   -0.134    -0.619    1.858    16.316   -4.164   -22.374
       tx16   -1.950   -25.040    2.236    10.662    2.542    25.366    0.927    16.333
       tx21   -0.593    -2.552   -4.388   -13.416   -1.258    -8.857   -2.122   -22.090
       tx22   -4.042*  -46.559   -0.761    -3.237    5.074*   56.706   -0.019    -0.644
       tx38    1.221     8.412   -4.675   -18.205   -0.266    -2.226   -3.939*  -33.442
       tx56   -0.330    -3.287   -5.151   -19.739    0.558     3.882   -2.310*  -32.595
       ut01   -1.703*  -76.230   -2.355   -13.422    0.563     3.662   -4.906   -32.675
       wa14   -0.773   -12.900   -0.869   -15.425    0.864*   77.984   -3.469   -16.795
       wa19   -3.779*  -29.212   -2.347   -25.188    1.733    35.108   -1.652   -25.456
       wa21   -2.120   -14.526   -3.788   -25.376    1.028    18.366   -7.923*  -57.686
       wy02   -4.968*  -42.674   -9.021*  -51.257   -0.740    -7.125   -2.037*  -58.345
       wy06    1.099    12.152   -2.555   -17.916    3.794*   37.058   -1.066*  -30.218
       wy08   -2.397*  -35.271    0.911    12.282    3.876*   69.203   -0.504   -18.702
       wy99   -1.812   -20.584   -4.699*  -26.039    0.157     1.137   -0.997*  -37.450
---------------------------------------------------------------------------------------
* Annual trend was significant (p<0.05).
----------------------------------------------------------------------------------------------------------

                 Ammonium            Calcium           Magnesium          Potassium            Sodium
             _________________  _________________  _________________  _________________  _________________
              Change   Percent   Change   Percent   Change   Percent   Change   Percent   Change   Percent
Region Site   (µeq/L)  Change    (µeq/L)  Change    (µeq/L)  Change    (µeq/L)  Change    (µeq/L)  Change
----------------------------------------------------------------------------------------------------------
 NE    il11    4.674*   27.414   -2.387*  -23.531   -0.615*  -26.888   -0.102   -21.469    0.118     5.102
       il18    5.905    27.732   -3.194   -24.840   -1.302*  -31.609   -0.043    -7.140    0.035     1.395
       il19    0.158     0.699   -4.139   -26.478   -0.888   -16.701   -0.232*  -31.375   -0.305    -8.764
       il35    0.868     7.234   -2.127*  -25.698   -0.638*  -31.277   -0.149   -28.119   -0.566   -17.113
       il63   -0.526    -3.614   -2.185*  -25.717   -0.786*  -37.004   -0.158   -24.569   -0.651   -17.027
       in20   -3.023   -13.513   -4.268*  -36.526   -1.961*  -48.948   -0.325*  -52.647   -1.252*  -39.147
       in22    8.674*   86.438    1.475    18.728   -0.104    -5.015   -0.003    -0.461   -0.987   -27.560
       in34    0.628     3.019    1.669     9.177   -0.120    -2.106   -0.237*  -36.766   -0.589   -18.913
       in41   -1.937    -8.641   -3.754*  -30.817   -1.271*  -35.023   -0.257*  -41.500   -0.524   -17.423
       ky03    2.171    19.998   -2.503*  -37.977   -0.549   -31.109   -0.012    -2.859   -0.652   -20.833
       ky22   -0.145    -1.757   -6.784*  -62.241   -1.524*  -65.390   -0.243*  -45.078   -0.769*  -29.903
       ky35    0.107     0.925   -2.850*  -33.793   -1.096*  -50.500    0.177    29.617   -0.553   -22.077
       ky38    4.537*   56.345   -0.866   -15.671   -0.571*  -32.758    0.050     9.981   -0.263    -7.185
       ma01    1.570    27.261   -0.724   -13.167   -0.463    -3.007   -0.167   -10.258    0.778     1.220
       ma08    2.241    27.662   -0.827*  -28.464   -0.672*  -34.050   -0.084   -23.411   -0.176    -3.654
       ma13    1.870    28.328   -0.324    -8.912   -1.290*  -32.103   -0.027    -5.170   -1.582   -11.652
       md03    4.531*   37.156   -2.255*  -35.655   -1.385*  -49.046   -0.175   -29.797   -2.130*  -35.515
       md13    1.060     8.371   -1.610*  -33.569   -1.304*  -36.385   -0.114   -19.776   -1.453   -14.631
       me00    1.230    19.663   -0.953   -21.259   -1.023*  -58.634   -0.146*  -36.784   -0.727   -19.867
       me02    2.602    44.733   -0.492   -19.787   -0.850*  -46.891    0.050    14.192   -1.447   -27.818
       me09    0.607    10.463   -0.969*  -36.060   -0.662*  -50.336   -0.090*  -27.650   -0.361   -13.328
       mi09   -0.163    -0.959   -1.685   -18.689   -1.074*  -36.394   -0.182*  -31.617   -0.188   -10.148
       mi26    0.150     0.712   -2.620*  -25.696   -1.145*  -34.168   -0.075   -15.713   -0.430   -16.865
       mi53    4.231    22.535   -1.539   -13.873   -0.834   -20.695   -0.147*  -27.070   -0.042    -1.843
       mi98    1.861    10.658   -1.955   -23.807   -1.124*  -40.958   -0.054   -13.227   -0.556   -25.885
       mi99    1.991    15.330   -2.135*  -26.778   -1.260*  -48.488   -0.247*  -41.220   -0.655*  -27.325
       nh02    0.939    11.658   -0.960*  -31.642   -0.701*  -46.503   -0.104*  -29.191   -0.383   -12.299
       nj99    3.177    31.440   -1.576*  -32.497   -1.523*  -41.783   -0.216*  -40.173   -0.902   -10.602
       ny08    0.314     1.722   -2.286*  -31.958   -1.146*  -48.192   -0.195*  -47.981   -0.478   -21.063
       ny10   -3.869*  -20.248   -2.486*  -32.200   -1.060*  -44.090   -0.521*  -67.629   -0.976*  -34.137
       ny20    0.376     3.781   -1.735*  -37.876   -0.904*  -56.959   -0.197*  -52.294   -0.429   -23.195
       ny52   -0.426    -2.240   -2.282*  -28.817   -1.087*  -42.022   -0.312*  -47.026   -0.749*  -25.443
       ny65    1.129     9.464   -1.483*  -30.536   -0.931*  -53.182   -0.118*  -38.293   -0.554*  -27.270
       ny68    2.864    32.375   -0.570   -17.146   -0.634*  -39.878    0.007     2.126    0.096     3.858
       ny98   -0.749    -7.017   -1.087*  -27.734   -0.806*  -53.095   -0.031    -8.635   -0.041    -3.057
       ny99    1.161    12.369   -1.361*  -30.306   -1.276*  -40.175    0.011     2.300   -0.760   -11.064
       oh09    2.857    21.114   -0.491    -7.099   -0.597   -26.799    0.183    47.570   -0.125    -4.848
       oh17    2.936    16.070   -3.119*  -31.490   -1.239*  -37.316   -0.065   -11.273   -0.348   -12.305
       oh49    0.304     2.140   -2.212*  -24.180   -1.078*  -37.099   -0.007    -1.022   -0.315   -12.103
       oh71   -0.209    -0.981   -1.599   -17.660   -0.857*  -30.188   -0.101   -21.977   -0.070    -2.909
       pa15   -0.626    -4.647   -2.632*  -40.102   -0.977*  -48.572   -0.113   -24.685   -0.685*  -27.393
       pa29   -0.158    -1.145   -1.043   -18.155   -0.670*  -37.015   -0.014    -3.392   -0.268   -12.984
       pa42   -1.175    -7.733   -1.653*  -27.257   -0.873*  -42.297   -0.251*  -39.487   -0.664*  -25.405
       pa72    0.779     7.871   -1.613*  -35.395   -0.925*  -41.267   -0.273*  -46.665   -0.205    -4.627
       va00    0.573     5.304   -1.398*  -33.741   -0.807*  -37.584   -0.324*  -45.391   -0.027    -0.600
       va13    1.894    21.329   -1.707*  -26.732   -1.046*  -45.720   -0.043    -4.394   -0.408   -13.750
       va28    0.282     2.805   -1.249*  -38.936   -0.869*  -57.856   -0.092   -25.859   -1.111*  -36.749
       vt01    1.075     9.732   -0.288    -5.850   -0.794*  -36.488   -0.148*  -29.853    0.232     8.135
       vt99    1.429    12.936   -0.876   -20.920   -0.806*  -51.355   -0.033    -9.622    0.011     0.659
       wi28   -1.147    -4.921   -4.743*  -37.595   -1.638*  -47.201   -0.379*  -47.855   -0.690*  -25.411
       wi36    2.104    15.145   -3.025*  -32.067   -1.266*  -48.088   -0.213*  -44.411   -0.516   -27.106
       wi37    0.455     2.185   -2.364   -20.894   -1.275*  -42.469   -0.372*  -51.688   -0.603*  -25.567
       wi99    0.140     0.605   -3.916*  -28.983   -1.438*  -32.628   -0.185   -26.339   -0.693   -25.593
       wv04   -1.344   -13.254   -2.690*  -46.311   -1.058*  -59.258   -0.344*  -49.726   -0.849*  -35.994
       wv18    1.696    15.546   -1.013   -13.406   -0.782*  -41.271   -0.144*  -24.443   -0.322   -15.786
       ---------------------------------------------------------------------------------------------------
 SE    al10   -1.632   -21.745   -3.704*  -55.514   -1.286*  -47.803   -0.371*  -42.285   -2.018*  -26.042
       al99    2.090    18.816   -1.580   -32.533   -0.679*  -34.585   -0.136   -20.876   -0.018    -0.384
       fl03    0.684    14.167   -1.780*  -31.372   -1.299*  -32.161   -0.414*  -48.448   -2.126   -14.455
       fl11    2.587*   73.907   -1.173   -17.180    0.402     5.714    0.328    23.489    3.528    12.892
       fl14   -0.024    -0.555   -1.492*  -38.360   -0.589   -19.598   -0.034    -5.985    1.255    14.342
       fl41    1.652    33.927   -1.707   -25.730   -1.270   -25.854   -0.269   -30.368   -1.461    -8.555
       ga20    0.913    12.524   -2.300*  -45.920   -0.677   -23.146    0.114    12.246    0.690     8.631
       ga41    0.899    12.120   -2.375*  -52.124   -1.068*  -45.527   -0.074    -9.528   -1.601*  -24.916
       ga50    0.889    15.527   -1.942*  -42.928   -0.730   -25.636    0.010     0.948   -1.367   -16.216
       ms10    1.898    23.161   -1.355   -28.909   -0.876*  -35.528   -0.389*  -42.162   -1.670   -22.396
       ms30    0.605     8.169   -0.763   -18.502   -0.826*  -40.308   -0.303   -38.026   -1.462   -26.526
       nc03    1.166    13.630   -1.982*  -46.498   -1.330*  -34.836   -0.163   -21.583   -2.280   -18.918
       nc25   -1.389   -16.315   -1.779*  -47.294   -0.590*  -38.738   -0.141   -24.792   -0.145    -3.706
       nc34   -1.028    -7.306   -2.147*  -44.188   -0.831*  -34.526   -0.216   -21.255    0.565    10.819
       nc36    3.495*   54.497   -0.621   -18.334   -0.471   -18.002   -0.116   -20.059    0.759     9.229
       nc41    3.960    31.576   -1.718*  -43.385   -1.069*  -35.603   -0.039    -4.733   -1.612   -18.766
       sc06    3.565*   89.764   -0.977   -19.852    0.145     4.836    0.990*  116.953   -0.299    -2.756
       tn00    1.288    14.157   -3.676*  -51.601   -1.420*  -60.232   -0.272*  -42.549   -0.928*  -24.703
       tn11   -1.671   -16.984   -2.294*  -43.676   -1.090*  -58.983   -0.634*  -57.495   -0.303   -11.886
       tn14    2.990*   42.675   -0.119    -3.206   -0.658*  -37.558   -0.065   -12.828   -0.862   -19.201
----------------------------------------------------------------------------------------------------------
* Annual trend was significant (p<0.05).

----------------------------------------------------------------------------------------------------------
                 Ammonium            Calcium           Magnesium          Potassium            Sodium
             _________________  _________________  _________________  _________________  _________________
              Change   Percent   Change   Percent   Change   Percent   Change   Percent   Change   Percent
Region Site   (µeq/L)  Change    (µeq/L)  Change    (µeq/L)  Change    (µeq/L)  Change    (µeq/L)  Change
----------------------------------------------------------------------------------------------------------
 West  ak03    0.328    22.307   -0.652   -35.275   -0.402*  -53.735   -0.110   -34.060   -0.272   -17.471
       ar02    1.458    14.340   -2.144*  -34.873   -0.419   -18.890    0.048     4.878    0.982    18.368
       ar03    2.088    23.465   -0.856   -14.285   -0.336   -16.402    0.276*   45.148    0.347     6.398
       ar16   -1.151   -10.280   -3.476*  -43.385   -0.865*  -42.478   -0.225   -26.454   -0.757   -18.101
       ar27   -1.447    -9.132   -3.534*  -35.058   -0.689*  -33.995   -0.082   -10.954   -0.819   -18.803
       az03    2.367    39.932   -6.629   -37.358   -2.424*  -43.227   -0.218   -35.780   -1.309   -29.331
       az06   -1.984   -12.857   -2.191   -16.500   -1.611   -25.943   -0.151   -13.495   -1.409    -8.329
       az99    2.799    32.489   -0.314    -3.428   -1.092*  -43.685    0.003     0.456    0.039     1.002
       ca42   -1.528    -9.797   -3.529*  -47.599   -2.101   -44.839   -0.363*  -47.752   -1.059    -8.048
       ca45    1.018    40.472   -1.392*  -52.769   -1.434*  -48.871   -0.254*  -49.151   -2.521   -26.673
       ca75   12.004    79.377   -1.243   -27.032   -0.952*  -47.407   -0.377   -28.800   -0.807   -20.414
       ca88   11.456*   30.744   -4.517*  -52.938   -2.493*  -46.582   -0.396   -30.909   -2.117   -25.024
       ca98    0.589     6.373   -7.116*  -67.043   -2.098*  -71.489   -0.265   -30.565   -2.858   -46.962
       ca99    3.388    28.336   -2.766   -39.983   -1.286*  -48.316   -0.254   -32.975   -1.504   -33.318
       co00    1.956    18.505   -6.674*  -48.434   -1.810*  -66.850   -0.400*  -43.074   -2.083   -35.954
       co01   10.121*   62.536   -3.479   -20.176   -1.329*  -44.684   -0.656   -42.711   -0.675   -17.075
       co02    4.691    88.297   -0.972   -12.748   -0.601   -32.111   -0.283   -37.214   -0.715   -23.569
       co15    2.140    34.196   -5.059*  -38.244   -1.829*  -53.014   -0.270*  -41.167   -1.193*  -35.769
       co19    3.975*   45.237   -2.310   -24.277   -1.300*  -54.610   -0.160   -17.780   -0.978*  -35.681
       co21    4.395*   62.489   -2.726   -26.850   -1.507*  -52.697   -0.520*  -50.061   -0.568   -23.138
       co22    2.022    10.012   -5.045*  -43.863   -1.795*  -65.640   -0.213   -31.164   -1.331*  -43.660
       co97    4.546*  162.938    0.719    13.715   -0.469   -29.992    0.066    17.290    0.506    33.869
       co98   -0.176    -2.718   -4.188*  -45.553   -1.306*  -58.458   -0.224*  -38.837   -0.577   -24.534
       co99    1.084    19.604   -4.882   -26.272   -1.198*  -35.450   -0.181*  -32.469   -0.231    -8.508
       ia08   10.961*   51.770    0.562     3.310   -0.182    -3.918   -0.158   -15.864   -0.258   -12.483
       ia23   14.272*   91.988   -0.600    -4.208   -0.513   -21.663   -0.106   -15.481   -0.314   -13.410
       id03    8.595*  110.849   -4.522   -39.011   -1.662*  -57.385   -0.318*  -45.363   -1.170   -29.323
       id11    7.950*  112.733   -1.298   -13.703   -1.249*  -46.534   -0.155   -17.302    1.140    23.453
       id15    3.735*  101.459    0.539    13.784   -0.055    -5.476    0.128    31.874    0.365    13.609
       ks07    4.372    34.134   -1.488   -12.421   -0.805*  -37.164   -0.303   -39.414   -0.986   -26.294
       ks31    5.264*   30.332   -0.593    -3.911   -0.739*  -29.990   -0.157   -22.125   -0.622   -20.846
       ks32   12.420*   62.339   -0.294    -2.182   -0.918   -37.936   -0.300   -25.542   -0.430   -17.641
       la12   -0.211    -1.964   -0.941   -18.245   -1.070*  -26.236   -0.239*  -28.499   -3.070   -19.900
       la30   -2.150   -18.954   -2.055*  -41.947   -1.258*  -35.659   -0.268*  -35.708   -2.628   -21.228
       mn16   -3.341   -18.045   -3.458*  -34.738   -1.153*  -42.180   -0.358*  -43.055   -1.188*  -46.631
       mn18   -0.398    -3.237   -3.411*  -43.475   -1.496*  -62.400   -0.342*  -58.788   -0.960*  -47.633
       mn23    8.736*   50.275   -1.483   -16.092   -0.730   -28.868   -0.201   -32.288   -0.271   -16.138
       mn27   -0.829    -2.563   -5.957*  -35.064   -2.434*  -48.721   -0.477*  -43.761   -0.922*  -34.723
       mo03    0.541     3.577   -2.969   -26.316   -0.683*  -29.106   -0.295*  -38.390   -0.602   -17.290
       mo05    0.912     7.419   -2.791*  -38.128   -1.039*  -44.084   -0.227   -24.301   -0.716   -17.229
       mt00    5.280*   94.964   -3.271   -32.278   -1.659*  -54.788   -0.220   -32.171   -1.136   -37.600
       mt05    0.715    19.846   -1.740*  -37.099   -0.743*  -51.972   -0.136   -20.378   -0.507   -23.756
       mt07    1.354    32.445   -1.739   -26.931   -1.218*  -64.684   -0.267*  -46.368   -1.023*  -44.767
       mt13    7.190*   76.482   -7.390   -46.012   -3.477*  -60.288   -0.482*  -51.669   -0.758   -17.550
       nd07    0.103     0.785   -4.454*  -37.191   -1.392*  -39.947   -0.200   -32.814   -0.687   -22.392
       nd08    6.749    33.177   -4.528*  -33.380   -1.214   -28.789   -0.180   -21.257   -0.758   -29.027
       nd11    7.878    34.468   -7.261   -36.445   -4.357*  -54.437   -1.068*  -51.747   -2.284*  -50.050
       ne15    0.610     1.795   -2.399   -15.079   -1.037*  -36.077   -0.233*  -27.478   -0.791   -27.844
       nm07    1.485    22.145   -5.494*  -39.985   -1.412*  -59.548   -0.580*  -64.803   -1.780*  -51.614
       nm08    4.683*   88.198   -1.762   -10.553   -1.276*  -45.323   -0.192   -34.113   -1.564   -39.808
       nm09    1.992    32.916   -4.118*  -38.062   -1.307*  -57.385   -0.256*  -44.626   -0.865*  -28.643
       nm12   10.147*  224.953   -0.199    -2.068   -1.145*  -51.085    0.128    24.588    0.325    14.177
       ok00    4.544    27.750   -6.887   -38.156   -1.875*  -54.064   -0.146   -16.327   -3.262*  -45.700
       ok17    0.497     3.418   -2.082   -15.025   -0.552   -20.181    0.317    41.094   -0.550   -12.740
       or02    0.417    28.398   -1.051*  -36.163   -2.589*  -37.916   -0.197   -24.536   -8.796   -31.331
       or09    2.639*  113.339   -0.863   -25.149   -0.616*  -46.120   -0.855*  -71.537   -1.742*  -46.888
       or10    0.167     9.871   -1.001*  -48.060   -0.893*  -44.136   -0.140*  -35.345   -1.477   -21.612
       or18    2.296*  107.112   -1.364*  -42.941   -0.549*  -54.986   -0.122   -27.152   -0.546   -23.875
       or97    3.260*  112.484   -1.356*  -42.919   -1.216*  -33.400   -0.110   -16.675   -0.526    -4.270
       or98    2.381*   66.291   -0.538*  -22.880   -0.769   -24.052   -0.048    -7.626   -0.782    -6.306
       sd08    2.320    16.011   -2.963   -31.685   -1.124*  -52.757   -0.338*  -48.856   -0.389   -17.798
       sd99    9.025    38.663   -2.069   -15.874   -0.921   -25.278   -0.203   -29.007   -0.119    -5.400
       tx03    8.123    70.118   -4.154   -29.400   -1.107   -18.793   -0.026    -2.052   -1.649    -7.954
       tx04    5.146    61.442   -3.723   -13.984   -1.231*  -47.204   -0.174   -21.954   -0.184    -4.448
       tx10    3.686    43.378   -3.257   -38.243   -1.472*  -32.417    0.097    11.714   -2.828   -18.539
       tx16    6.581*   74.111    4.647    33.808   -0.255   -10.896    0.076    11.633    0.832    14.546
       tx21   -1.024   -10.358   -3.471*  -39.886   -1.068*  -34.480   -0.182   -19.349   -1.800   -20.602
       tx22    6.660*   88.288    5.972    40.371   -0.148    -6.026    0.139    29.157   -0.065    -1.963
       tx38   -1.244   -11.390   -3.752*  -44.423   -1.685*  -44.372   -0.867*  -44.249   -3.553*  -33.073
       tx56    3.767    28.864   -7.207*  -37.756   -1.391*  -46.932   -0.300   -32.801   -2.791*  -39.362
       ut01   11.967    33.625    1.038     6.788   -0.805   -18.320   -0.163   -21.373   -1.301   -12.301
       wa14    0.100     8.027   -0.685*  -36.362   -1.015   -24.032   -0.091   -17.296   -0.295    -1.879
       wa19    1.032*   57.147   -0.713*  -41.248   -1.094*  -52.413   -0.000    -0.065   -0.174    -3.945
       wa21    1.445    58.465   -1.579*  -57.388   -2.108*  -65.664   -0.067   -14.033   -6.561*  -55.343
       wy02    0.927    16.481   -6.862*  -54.802   -2.632*  -72.074   -0.242*  -50.588   -1.657*  -51.023
       wy06    3.034*   58.344   -3.709   -32.863   -1.872*  -59.954   -0.284*  -49.033   -1.229   -32.334
       wy08    4.795*  113.937    0.745     9.152   -0.704   -33.909   -0.199   -28.406    0.471    24.535
       wy99    2.861    31.035   -3.790   -25.688   -1.785*  -55.638   -0.299*  -42.363   -1.723*  -52.391

* Annual trend was significant (p<0.05).

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Last Update: 1536 08JUL96 kjl