Complex crystal cargo in basaltic eruptions has the potential to yield diverse insights on pre- and syn-eruptive timescales of magma storage and transport. Research on eruption products from the 1959 eruption from Kīlauea Iki Crater at Kīlauea volcano (Hawai‘i) demonstrates that time-series samples collected during an eruption can yield a wealth of information not accessible by studying the fall deposit alone. Major element zoning in olivine crystals illustrates four environments of magma storage that were variably mixed and progressively involved in the eruption. Diffusion timescales retrieved from crystals < 1 mm in size are typically much shorter than those from crystals > 1 mm, illustrating the additional complexity of information recorded by different grain sizes and olivine populations. The timescales can be divided into two groups: (1) t > 100 days reflect longer-term magma recharge into Kīlauea’s deep (8–10 km) reservoir system and (2) t < 100 days broadly correspond to a period of unrest and inflation beginning ~ 3 months prior to eruption. Some timescales reflect syn-eruptive processes, where diffusion began after the eruption onset. Progressive changes in zoning populations in the time-series scoriae samples illustrate how quickly diffusive re-equilibration can erase older magmatic histories and information and underscores that studies on fall deposits can lead to an incomplete record of magmatic processes. Thus, diffusion timescales from fall deposits alone should be cautiously interpreted with the caveat that they may be missing a substantial part of the total eruptive event and, therefore, the record of magmatic histories inferred from crystal cargo.