Excessive fine-grained sediment runoff due to anthropogenic activities is a major environmental concern for watersheds worldwide, especially so for urban areas such as Washington, D.C. Dated grey infrastructure, i.e., the network of buried pipes and reservoirs managing water resources, can amplify existing issues with sediment runoff and associated pollutants. This infrastructure, which is generally designed to quickly transport stormwaters away from urban areas, contributes to urban stream syndrome. Recent studies have suggested aging subterranean infrastructure may be an unaccounted-for source of sediments. The composition of this possible sediment source, and the extent to which it contributes to urban sediment runoff, is poorly understood. Our study seeks to examine sediment sources and transport processes in an urban watershed with an entirely buried drainage network using sediment fingerprinting, with specific attention paid to differentiating between terrestrial and subterranean sources. We demonstrate here multiple novel approaches to sampling subterranean sources including augering and entering the buried drainage network itself. The results of this study may inform sediment managers and infrastructure engineers and allow for targeted sediment reduction responses.