The Imbrium basin is one of the largest and youngest impact basins on the Moon. It has experienced multiple phases of volcanism that filled the basin with basaltic lavas, obscuring most evidence of geologic activity prior to the emplacement of mare basalts. Elevated basin ring massifs, however, can retain some of that history due to their higher topographic elevation compared to the maria. In this work, we use thermal infrared and radar data sets in conjunction with compositional data sets to establish the presence of external material that has been deposited on top of several remnant basin massifs of Imbrium. These massifs originally formed as part of the Imbrium basin ring structure, but their material properties indicate that they have since experienced modification from outside sources. In southwest Imbrium, we present evidence that Mons Vinogradov was mantled by rock-poor, glassy pyroclastic material prior to the deposition of Eratosthenian-era basalts immediately surrounding the mons. In northern Imbrium, we find that Montes Recti and Montes Teneriffe were not affected by pyroclastic volcanism but rather were mantled by rock- and glass-poor ejecta materials likely related to the Iridum basin impact. At Mons Piton in eastern Imbrium, we see weaker glass signatures than those found at Mons Vinogradov, which we suggest could be due to a thin layer of reworked or partially buried glassy pyroclastic material. These results indicate that basin ring massifs provide a mechanism for studying the geologic history of lunar impact basins.